基于等参梯度单元分析界面层属性对石墨烯/环氧树脂复合材料弹性性能的影响

Effects of interfacial layer properties on elastic properties of graphene/epoxy composites based on isoparametric graded element

  • 摘要: 针对石墨烯片在环氧树脂基体内定向连续和定向非连续分布的复合材料,通过分别构建三明治代表体单元和嵌入式代表体单元,进行了弹性性能预测的研究。代表体单元是三相复合结构,其中石墨烯和环氧树脂基体之间的界面层视为连续介质,其材料属性分别考虑均匀、线性和指数变化等3种情况。在代表体单元的有限元建模过程中,石墨烯和环氧树脂基体分别采用梁单元和实体单元进行离散,而界面层则采用等参梯度单元逼近。采用有限元软件ABAQUS 分析了小应变下的代表体单元的力学变形行为并提取其弹性性能,然后分析了界面层属性对石墨烯/环氧树脂复合材料弹性性能的影响。通过与混合率模型、修正的Halpin-Tsai模型及实验数据对比,验证了本文提出的基于等参梯度单元计算方法的有效性。数值算例表明,在处理界面层材料属性不均匀分布的问题方面,等参梯度单元具有计算量少、收敛快和精度高的优点。石墨烯/环氧树脂复合材料杨氏模量预测结果显示,界面层材料属性采用梯度变化的模型时,杨氏模量计算结果比均匀分布的模型、混合率模型和修正的Halpin-Tsai模型的结果偏大,但是更接近实验值。本文的研究结果说明界面层属性是影响复合材料力学性能的重要因素,并为寻求复合材料力学性能更精确地分析提供有效的途径。

     

    Abstract: The elastic properties of the composites with graphene sheets distributed continuously and discontinuously in the epoxy matrix were investigated via sandwich representative volume element (RVE) and embedded RVE, respectively. The RVEs were considered as a three phase composite structure, in which the interphase between graphene and epoxy resin matrix was treated as continuum medium while its material properties were considered to vary uniformly, linearly and exponentially. In the finite element modeling process of the RVE, the graphene was discretized using beam element and the epoxy matrix was discretized via the use of solid element while the interfacial layer was approached using isoparametric graded element (IGE). The finite element software ABAQUS was used to analyze the mechanical deformation behavior of the RVE subjected to small strains and extract its elastic properties. The extracted results of elastic properties were then used to study the effects of interfacial layer properties on the elastic properties of graphene/epoxy composites. The validity of the proposed computational method based on the IGE was verified by comparing with rule of mixture (ROM), the modified Halpin-Tsai model and the experimental data. Numerical examples illustrate that the IGE has the advantages of less computation, fast convergence and high accuracy in dealing with the uneven distribution of material properties in the interfacial layer. The prediction results of Young's modulus of composites reveal that when the material properties of interfacial layer adopt the gradient model, the calculated results of Young's modulus are larger than those of uniform distribution model, ROM and the modified Halpin-Tsai model, but closer to the experimental value. The results of this research show that the property of interfacial layer is an important factor affecting the mechanical properties of composites, and provide an effective way to seek more accurate analysis of the mechanical properties of composites.

     

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