无胶秸秆基纤维板的研究进展

苏琼; 卢新宇; 石小琴; 聂宏杰; 张平; 王彦斌

doi:10.13801/j.cnki.fhclxb.20230907.002

无胶秸秆基纤维板的研究进展

doi: 10.13801/j.cnki.fhclxb.20230907.002

苏琼^{1, 2, 3, 4},
卢新宇^{1, 2, 3, 4},
石小琴^{1, 2, 3, 4},
聂宏杰^{1, 2, 3, 4},
张平¹,
王彦斌^{1, 2, 3, 4, ,}

1.
西北民族大学　化工学院，兰州 730030
2.
环境友好复合材料国家民委重点实验室，兰州 730030
3.
甘肃省生物质功能复合材料工程研究中心，兰州 730030
4.
甘肃省高校环境友好复合材料及生物质利用重点实验室，兰州 730030

基金项目: 国家自然科学基金(21968032；22165025)；甘肃省科技计划项目(20YF8FA045)；中央高校基本科研业务费项目(31920220044；31920230003；31920230022；31920230023)；西北民族大学化学学科创新团队(1110130139；1110130141)；省级一流专业建设(2019SJYLZY-08)；甘肃省高校创新创业教育改革项目(2021SJCXCYXM-01；2021SJCXCYTD-01)

详细信息

通讯作者:
王彦斌，博士，教授，博士生导师，研究方向为生物质复合材料　E-mail: ybwang@126.com

中图分类号: TQ35；TB332
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- 文章访问数: 357
- HTML全文浏览量: 194
- PDF下载量: 25
- 被引次数: 0
出版历程
- 收稿日期: 2023-06-27
- 修回日期: 2023-08-23
- 录用日期: 2023-08-25
- 网络出版日期: 2023-09-08
- 刊出日期: 2024-04-15

Research progress of glue-free fiberboard based on straw

SU Qiong^{1, 2, 3, 4},
LU Xinyu^{1, 2, 3, 4},
SHI Xiaoqin^{1, 2, 3, 4},
NIE Hongjie^{1, 2, 3, 4},
ZHANG Ping¹,
WANG Yanbin^{1, 2, 3, 4
, ,}

1.
School of Chemical Engineering, Northwest Minzu University, Lanzhou 730030, China
2.
Key Laboratory of Environment-Friendly Composite Materials of the State Ethnic Affairs Commission, Lanzhou 730030, China
3.
Gansu Provincial Biomass Functional Composite Materials Engineering Research Center, Lanzhou 730030, China
4.
Key Laboratory of Utility of Environmental Friendly Composite Materials and Biomass in Universities of Gansu Province, Lanzhou 730030, China

Funds: National Natural Science Foundation of China (21968032; 22165025); Gansu Provincial Science and Technology Program (20YF8FA045); Central Universities' Basic Scientific Research Expenses Program (31920220044; 31920230003; 31920230022; 31920230023); Northwest Minzu University Innovation Team in Chemistry Discipline (1110130139; 1110130141); Provincial First-class Professional Construction (2019SJYLZY-08); Gansu Provincial Universities Innovation and Entrepreneurship Education Reform Program (2021SJCXCYXM-01; 2021SJCXCYTD-01)

摘要

摘要: 无胶秸秆基纤维板是生物质复合材料，具有无毒、可降解、可回收和可再生等特点。因其不消耗石油资源，有利于可持续发展，可替代部分木材应用于地板、建筑材料、家具、室内装修等领域。但对其制板机制及工艺的研究较欠缺，导致市场份额占比仍较低。本文综述了无胶秸秆基纤维板的自粘结机制和应用现状，分析了近年来无胶秸秆基纤维板的工艺进展，着重从纤维的预处理、纤维尺寸、工艺参数(压制时间、压力和温度)对无胶秸秆基纤维板性能的影响进行了系统综述，并对未来无胶秸秆纤维板的优化设计、大规模生产及推广应用进行了展望。
- 无胶秸秆基纤维板 /
- 生物质 /
- 自粘结机制 /
- 制造工艺 /
- 秸秆预处理
Abstract: Glue-free straw-based fiberboard is a biomass composite material, which is nontoxic, degradable, recyclable and renewable. As it does not consume petroleum resources, it is conducive to sustainable development, and can replace some wood used in fields such as flooring, building materials, furniture and interior decoration. However, there is a lack of research on its board making mechanism and process, resulting in a still low market share. In this paper, the self-bonding mechanism and application status of glue-free straw-based fiberboard are summarized. The technological progress of glueless straw-based fiberboard in recent years is introduced. The effects of fiber pretreatment, fiber size and process parameters (such as pressing time, pressure and temperature) on the performances of glueless straw-based fiberboard are systematically discussed. The future prospect of glueless straw-based fiberboard in optimal design, industrial production and promotion on a large scale are put forward.
- glue-free straw-based fiberboard /
- biomass /
- self-bonding mechanism /
- manufacturing process /
- pretreatment of straw

HTML全文

图 1 自由基聚合的反应机制^[13]

Figure 1. Reaction mechanism of free radical polymerization^[13]

下载: 全尺寸图片幻灯片

图 2 无胶全纤维素纤维板的生产示意图^[22]

Figure 2. Schematic experimental procedure for the production of binderless all-cellulose fibreboard^[22]

RT—Room temperature

下载: 全尺寸图片幻灯片

图 3 无胶秸秆纤维板材的应用：((a)~(d)) 吸声纤维板；((e)~(h)) 墙体装饰纤维板

Figure 3. Application of glue-free straw fiberboard: ((a)-(d)) Acoustic fiberboard; ((e)-(h)) Wall decorative fiberboard

下载: 全尺寸图片幻灯片

表 1 秸秆类型及预处理方法对无胶秸秆纤维板性能的影响

Table 1. Effects of different raw materials and different pretreatments on the properties of glue-free straw fiberboard

Raw materials	Pretreatment classification	Pre-processing methods	Changes in board performance	Ref.
Corn straw	Chemical pretreatment	Alkaline treatment with 2% NaOH solution	MOR increased by 75.6%, MOE increased by 101.4%, IB increased by 75%, and TS decreased by 22% compared to no pretreatment	[16]
Rice straw		NaOH solution alkali treatment	The highest IB value of hot pressed straw board was obtained when the mass fraction of 1wt%NaOH pretreated straw fiber, and the mechanical properties of the board were poor when the NaOH content was greater than 1wt%	[28]
		Oxalic acid (OA) treatment	Compared with steam treatment, MOE and MOR were reduced by 9.9% and 8.6% respectively, and the mechanical properties of the board met ANSI standards	[31]
		Bis-(3-triethoxysilylpropyl) tetra sulphide (Si-69) pre-cured	With the increase of Si-69 concentration, both MOR and MOE of fiberboard tended to increase, and TS and WA decreased sharply	[32]
Wheat straw		Treatment with 10% H₂SO₄ followed by 4% H₂O₂	H₂SO₄ loosened the physical structure of straw, H₂O₂ reacted with the fiber surface and activated the fiber surface to make it self-bonding, which improved the mechanical properties of fiberboard	[33]
Triticale straw		Bleaching with sodium hypochlorite after treatment with sodium hydroxide pulping	Significantly lower hemicellulose content and enhanced board mechanical properties	[34]
Winter wheat hulls		2% NaOH solution treatment	The lignin content and equilibrium moisture content increased, the thickness expansion of the slab after pretreatment increased, and the mechanical properties of the board decreased	[35]
Jute straw		Alkali (NaOH) and alkali, silane	The crystallinity index of jute fibers treated with alkali silane was lower than that of alkali-treated jute fibers	[36]
Rice straw	Physical pretreatment	Steaming and hot grinding	Compared with OA treatment, the MOE and MOR of the board increased by 6.0% and 13.9% respectively, and the mechanical properties of the board were better than untreated	[37]
Giant reed straw		Steam blasting pretreatment	The best IB, MOE, MOR, WA and TS were 1.28 MPa, 7439 MPa, 40.4 MPa, 17.6% and 13.3%, respectively, and the fiberboards exceeded the requirements of the relevant standard specifications	[38]
Sugarcane straw		Steam blasting pretreatment	Compared to the NaOH pretreated material, the steam-exploded material had high tensile strength and high water resistance	[39]
Winter wheat hulls		Heat treatment (boiling water) and plasma treatment	Both can improve the surface energy of the shell, reduce the equilibrium moisture content of the shell, and improve the mechanical properties of the sheet	[35]
Coriander straw		Steam treatment and mechanical refining of twin-screw extruders	The material had good properties with a MOR of 29 MPa and a TS of 24%, and the water sensitivity of the plate had been reduced by 63%	[40]
Rape straw		Steam treatment	The tensile strength and modulus of elasticity of the fiberboard both increased significantly with the increase in cooking temperature, and at a cooking temperature of 200℃, the tensile strength was 0.014 MPa, the modulus of elasticity was 0.442 MPa, and the TS was 3.4%	[41]
Wheat straw	Enzymatic pretreatment	Enzyme treatment	The mechanical properties of enzyme-treated fiberboard were significantly higher than those of non-enzyme-treated semi-chemical pulp fiberboard, and had excellent bond strength	[3]
Wheat straw	Enzymatic pretreatment	Laccase pretreatment	Activation of the fiber surface, increase in the number of chemical bonding points between the fibers, increase in the mechanical properties of the board with longer incubation time of laccase	[24, 15]
Notes: MOR—Modulus of rupture; MOE—Modulus of elasticity; IB—Internal bonding; TS—Thickness swelling; WA—Water absorption; ANSI—American National Standards Institute.

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表 2 热压工艺对比

Table 2. Comparison of hot pressing process

Hot pressing process	Advantages and disadvantages	Application	Ref.
Continuous flat pressing method	Small thickness error, no sanding, small trimming loss, advanced technology, but large equipment and high primary cost	Preparation for reed straw fiber particle board	[53]
Roller press method	Economical, with good mechanical properties and water resistance, but only boards up to 1 cm thick can be prepared	High-performance wood scrimber prepared by a roller-pressing impregnation method	[54]
Multi-layer press flat pressing method	Suitable for the preparation of medium-thick plates, but the thickness error is large and the sanding area is large	Bonded bamboo panels	[55]

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