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新型碳基磁性复合吸波材料的研究进展

曹敏 邓雨希 徐康 郝晓峰 胡嘉裕 杨喜

曹敏, 邓雨希, 徐康, 等. 新型碳基磁性复合吸波材料的研究进展[J]. 复合材料学报, 2020, 37(12): 3004-3016. doi: 10.13801/j.cnki.fhclxb.20200825.002
引用本文: 曹敏, 邓雨希, 徐康, 等. 新型碳基磁性复合吸波材料的研究进展[J]. 复合材料学报, 2020, 37(12): 3004-3016. doi: 10.13801/j.cnki.fhclxb.20200825.002
CAO Min, DENG Yuxi, XU Kang, et al. Research progress of new carbon based magnetic composite electromagnetic waveabsorbing materials[J]. Acta Materiae Compositae Sinica, 2020, 37(12): 3004-3016. doi: 10.13801/j.cnki.fhclxb.20200825.002
Citation: CAO Min, DENG Yuxi, XU Kang, et al. Research progress of new carbon based magnetic composite electromagnetic waveabsorbing materials[J]. Acta Materiae Compositae Sinica, 2020, 37(12): 3004-3016. doi: 10.13801/j.cnki.fhclxb.20200825.002

新型碳基磁性复合吸波材料的研究进展

doi: 10.13801/j.cnki.fhclxb.20200825.002
基金项目: 中南林科大人才启动基金(2018YJ033);湖南省教育厅科研项目(18B173)
详细信息
    通讯作者:

    杨喜,博士,讲师,研究方向为生物质碳基功能材料 Email:yangxijy@126.com

  • 中图分类号: TB333

Research progress of new carbon based magnetic composite electromagnetic waveabsorbing materials

  • 摘要: 新型碳基磁性复合吸波材料因兼具质轻和高性能而成为当今电磁波吸收材料的研究主流。碳系吸波材料既有密度小、比表面大、电导率高等优点,也存在无磁性、阻抗匹配水平低等不足,常通过与磁损耗物质复合来构筑多样微结构、多元协同损耗机制的轻质复合材料,实现高强与宽频电磁波吸收。本文在总结国内外碳基复合材料吸波应用的研究基础上,以成分组成、复合方法、微观结构等为主线对比分析了新型石墨烯、碳纳米管、生物质多孔碳及其他碳系磁性复合吸波材料的研究进展,并指出了磁性碳系吸波材料存在的问题及未来发展趋势。

     

  • 图  1  FeCoNi/石墨烯(GR)微结构示意图和反射率曲线

    Figure  1.  Microstructure diagram and reflectivity curves of FeCoNi/graphene (GR)

    图  2  CoFe2O4((a)、(c))与还原氧化石墨烯(RGO)/CoFe2O4((b)、(d))的损耗因子及反射损耗值

    Figure  2.  Loss tangent and reflection loss of CoFe2O4 ((a), (c)) and reduced graphene oxide (RGO)/CoFe2O4((b), (d))

    图  3  碳纳米管(CNTs)/Fe3C的制备示意图

    Figure  3.  Preparation diagram of carbon nanotubes (CNTs)/Fe3C

    图  4  CoNi/N-GR掺杂CNTs的三维结构及吸波原理

    Figure  4.  3D structure and absorbing principle of the CoNi/N-GR doped CNTs

    图  5  Fe3O4/WC孔道特征及吸波性能

    Figure  5.  Pore characteristics and absorbing properties of Fe3O4/WC

    图  6  核壳Co@Co3O4/C复合材料的吸波原理

    Figure  6.  EM wave absorption mechanism of core-shell Co@Co3O4C composite

    图  7  Fe3O4-CNTs-空心多孔碳纤维(HPCFs)复合材料制备示意图

    Figure  7.  Schematic illustration of Fe3O4-CNTs-hollow porous carbon fibers (HPCFs) composites formation

    表  1  GR基磁性复合材料的吸波性能

    Table  1.   Wave absorption properties of GR based magnetic composites

    MaterialMethodRLmin/dBDm/mmBand width/GHzRef.
    NiFe2O4/RGO Hydrothermal method −42 5.3 [13]
    CoFe2O4/GR Vapor diffusion −18.5 2 3.7 [14]
    BaFe12O19/GA Chemical vapor deposition −18.35 2 3.32 [15]
    SGN/Fe3O4 Solvothermal route −41 2.0 5.3 [16]
    ZnCo2O4/C/MG Coprecipitation −52.9 4.48 3.9 [17]
    Fe3O4@SiO2−RGO Covalent modification −55.4 6.24 3.5 [18]
    ZnFe2O4@SiO2@RGO Heat treatment −43.9 2.8 6 [19]
    NiFe2O4@MnO2/GN Hydrothermal method −47.4 3 4.3 [20]
    Notes: GA—Graphene aerogel; SGN—S-doped graphene; MG—Magnetic graphene; GN—Graphene nanocrystals; RLmin, Dm—Minimum reflectivity and matching thickness, respectively.
    下载: 导出CSV

    表  2  铁氧体/CNTs复合材料的吸波性能

    Table  2.   Microwave absorbing properties of ferrite/CNTs composites

    MaterialMethodRLmin/dBDm/mmBand width/GHzRef.
    BaFe12O19/CNTs Chemical vapor deposition −21.5 2 2.5 [37]
    CoFe2O4/CNTs Chemical vapor deposition −18 6.5-13.5 [38]
    SrFe12O19/MWCNTs Sol-gel method −19.7 3 [39]
    BaFe12O19/ZnFe2O4/CNTs Autoignition method −43.22 2 2.95 [40]
    ZnFe2O4/MWCNTs Solvothermal method −55.5 1.5 3.6 [41]
    Fe3O4/MnO2/CNTs Solvothermal method −42.2 7.1 [42]
    Notes: CNTs—Carbon nanotubes; MWCNTs—Multi-wall carbon nanotubes.
    下载: 导出CSV
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  • 收稿日期:  2020-06-15
  • 录用日期:  2020-08-25
  • 网络出版日期:  2020-08-26
  • 刊出日期:  2020-12-15

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